This paper presents a new rapid, low-cost method for the large-scale documentation of pottery sherds through simultaneous multiple 3D model capture using Structure from Motion (SfM). The method has great potential to enhance and replace time-consuming and expensive conventional approaches for pottery documentation, i.e., 2D photographs and drawing on paper with subsequent digitization of the drawings. To showcase the method’s effectiveness and applicability, a case study was developed in the context of an investigation of the Phoenician economy at the Lebanese site of Tell el-Burak, which is based on a large collection of amphora sherds. The same set of sherds were drawn by an experienced draftsperson and then documented through SfM using our new workflow to allow for a direct comparison. The results show that the new technique detailed here is accessible, more cost-effective, and allows for the documentation of ceramic data at a far-greater scale, while producing more consistent and reproducible results. We expect that these factors will enable excavators to greatly increase digital access to their material, which will significantly enhance its utility for subsequent research.