Noncovalent van der Waals (vdW) interactions are responsible for a wide range of phenomena in matter. Popular density-functional methods that treat vdW interactions use disparate physical models for these intricate forces, and as a result the applicability of these methods is often restricted to a subset of relevant molecules and materials. Aiming towards a general-purpose density functional model of vdW interactions, here we unify two complementary approaches: nonlocal vdW functionals for polarization and interatomic methods for many-body interactions. The developed nonlocal many-body dispersion method (MBD-NL) increases the accuracy and efficiency of existing vdW functionals and is shown to be broadly applicable to molecules, soft and hard materials including ionic and metallic compounds, as well as interfaces between organic molecules and inorganic materials.
