dc.contributor.author
Tschannen, Cla Duri
dc.contributor.author
Frimmer, Martin
dc.contributor.author
Gordeev, Georgy
dc.contributor.author
Vasconcelos, Thiago L.
dc.contributor.author
Shi, Lei
dc.contributor.author
Pichler, Thomas
dc.contributor.author
Reich, Stephanie
dc.contributor.author
Heeg, Sebastian
dc.contributor.author
Novotny, Lukas
dc.date.accessioned
2021-11-09T12:54:46Z
dc.date.available
2021-11-09T12:54:46Z
dc.identifier.uri
https://refubium.fu-berlin.de/handle/fub188/32628
dc.identifier.uri
http://dx.doi.org/10.17169/refubium-32352
dc.description.abstract
We investigate the anti-Stokes Raman scattering of single carbyne chains confined inside double-walled carbon nanotubes. Individual chains are identified using tip-enhanced Raman scattering (TERS) and heated by resonant excitation with varying laser powers. We study the temperature dependence of carbyne’s Raman spectrum and quantify the laser-induced heating based on the anti-Stokes/Stokes ratio. Due to its molecular size and its large Raman cross section, carbyne holds great promise for local temperature monitoring, with potential applications ranging from nanoelectronics to biology.
en
dc.format.extent
7 Seiten
dc.rights.uri
https://creativecommons.org/licenses/by/4.0/
dc.subject
linear carbon chains
en
dc.subject
Raman scattering
en
dc.subject
Raman thermometry
en
dc.subject
nanometrology
en
dc.subject.ddc
500 Naturwissenschaften und Mathematik::540 Chemie::540 Chemie und zugeordnete Wissenschaften
dc.title
Anti-Stokes Raman Scattering of Single Carbyne Chains
dc.type
Wissenschaftlicher Artikel
dcterms.bibliographicCitation.doi
10.1021/acsnano.1c03893
dcterms.bibliographicCitation.journaltitle
ACS Nano
dcterms.bibliographicCitation.number
7
dcterms.bibliographicCitation.pagestart
12249
dcterms.bibliographicCitation.pageend
12255
dcterms.bibliographicCitation.volume
15
dcterms.bibliographicCitation.url
https://doi.org/10.1021/acsnano.1c03893
refubium.affiliation
Physik
refubium.resourceType.isindependentpub
no
dcterms.accessRights.openaire
open access
dcterms.isPartOf.eissn
1936-086X
refubium.resourceType.provider
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