dc.contributor.author
Ma, Lin
dc.contributor.author
Galstyan, Gegham
dc.contributor.author
Zhang, Keke
dc.contributor.author
Kloc, Christian
dc.contributor.author
Sun, Handong
dc.contributor.author
Soci, Cesare
dc.contributor.author
Michel-Beyerle, Maria E.
dc.contributor.author
Gurzadyan, Gagik G.
dc.date.accessioned
2018-06-08T03:16:37Z
dc.date.available
2015-09-10T05:36:04.400Z
dc.identifier.uri
https://refubium.fu-berlin.de/handle/fub188/14831
dc.identifier.uri
http://dx.doi.org/10.17169/refubium-19020
dc.description.abstract
The two-photon-induced singlet fission was observed in rubrene single crystal
and studied by use of femtosecond pump-probe spectroscopy. The location of
two-photon excited states was obtained from the nondegenerate two-photon
absorption (TPA) spectrum. Time evolution of the two-photon-induced transient
absorption spectra reveals the direct singlet fission from the two-photon
excited states. The TPA absorption coefficient of rubrene single crystal is 52
cm/GW at 740 nm, as obtained from Z-scan measurements. Quantum chemical
calculations based on time-dependent density functional theory support our
experimental data.
en
dc.rights.uri
http://publishing.aip.org/authors/web-posting-guidelines
dc.subject.ddc
500 Naturwissenschaften und Mathematik::530 Physik
dc.subject.ddc
500 Naturwissenschaften und Mathematik::540 Chemie
dc.title
Two-photon-induced singlet fission in rubrene single crystal
dc.type
Wissenschaftlicher Artikel
dcterms.bibliographicCitation
The Journal of Chemical Physics. - 138 (2013), 18, Artikel Nr. 184508
dcterms.bibliographicCitation.doi
10.1063/1.4804398
dcterms.bibliographicCitation.url
http://dx.doi.org/10.1063/1.4804398
refubium.affiliation
Biologie, Chemie, Pharmazie
de
refubium.mycore.fudocsId
FUDOCS_document_000000023088
refubium.resourceType.isindependentpub
no
refubium.mycore.derivateId
FUDOCS_derivate_000000005387
dcterms.accessRights.openaire
open access
